No. You can get his mask but that is all.
Well in a way you do. Its believed when William Black fought Jack of Blades he survived by putting his soul in his mask. Which means his body or "form" had been broken. So Jack's mask might have spoken to other heroes who put the mask on and it in a way killed them and they became Jack through the mask causing his soul to live on with the mask your evil is increased greatly and you cant take it off. Though in Fable II it turns out the Hero of Oakvale threw the mask in the lava and Jack so far seems finally dead.